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I. 有機金屬催化反應 II. 有機碟狀聯苯分子應用於E-型偏光片研發
Dissertation

I. 有機金屬催化反應 II. 有機碟狀聯苯分子應用於E-型偏光片研發

葉國良
Doctor of Philosophy (PHD), 國立清華大學, 化學系
2004

Abstract

過渡金屬 釕金屬 鋅金屬 催化 圓盤型分子 液晶 六聯苯 偏光膜 丙烯醇 紫外光譜 薄膜 環化 碳碳三鍵裂解 氫原子的轉移反應 transition metal ruthenium zinc catalyze disk-molecule liquid crystal hexa-peri-hexabenzocoronene HBC polarizer propargyl alcohol UV spectrum thin film cyclization C-C triple bond cleavage Transfer Hydrogen Reaction
Abstract Organometallics plays an essential role on organic synthesis in these decades. It was applied in coupling reactions, cyclization reactions or ring opening reactions. Organometallics catalyzed reactions not only have good regioselectivities but have good stereoselectivities. In natural products synthesis, it is very important to control stereo or regio direction in specific positions. We emphasize on ruthenium and zinc metal complex which apply in ethynyl alcohol catalyzed transfer reactions. First, ruthenium complex was applied on transformation of propargyl ether into 1,3-dienes and benzaldehyde via transfer hydrogen. Second, ruthenium complex was apply on cleavage of a carbon-carbon triple bond: efficient transformation of propargyl alcohols into alkenes and carbon monoxide. Last, we used zinc complex on cyclization from propargyl alcohols. These reactions worked on mild conditions and used less catalyst (5 %) without any other chemical reagents to complete the reactions. These new reactions chemistry is Green Chemistry. Liquid crystal display (LCD) was developed full of vitality during decades. Because of the O-type polarizer, one drawback of the LCD is the narrow of the view angel. Although compensation film can improve the view angle, it critically reduces the backlight and increases the cost. We synthesis disk molecules to apply in E-type polarizer. E-type polarizer not only can increase the view angel, but also reduce the cost.

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