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液相微萃取法於環境水樣及尿液之微量有機污染物分析方法之研究與開發
Dissertation

液相微萃取法於環境水樣及尿液之微量有機污染物分析方法之研究與開發

張景翔
Doctor of Philosophy (PHD), 國立清華大學, 化學系
2007

Abstract

液相微萃取 分散式液液微萃取 動態頂空單滴微萃取 鹵素醚類 安非他命 芳香胺 氣相層析 電子捕捉偵測器 火焰離子化偵測器 質譜儀 化學衍生 中空纖維 Liquid-phase microextraction Dispersive liquid -iquid microextraction Dynamic headspace single-drop microextraction Haloether Amphetamine Aromatic amine Gas-Chromatography Electron capture detector Flame ionization detector Mass Spectrometer Chemical Derivatization Hollow Fiber
Abstract The development of faster, simpler and economic sample-preparation techniques is an important issue in chemical analysis. In this work, four analytical methods base liquid-phase microextraction (LPME) and dispersive liquid-liquid microextraction (DLLME) were described. The developed methods have been applied to the analysis of trace pollutants and abuse drugs in different sample matrices such as lake, river or human urine. Liquid phase microextraction method, which included hollow fiber liquid-phase microextraction (HF-LPME), single-drop microextraction (SDME), were investigated in the chapter one, chapter two, and chapter four. This methodology provided to be extremely simple, low cost and virtually solvent-free sample-preparation technique, which provided a high degree of selectivity and enrichment. The results show that these sample-preparation coupled with GC-ECD or GC-MS could determinate the trace organic pollutants in the ppb level. The DLLME developed by Yaghoub Assadi in 2006 has emerged as a virtually time-free alternative for extraction time to conventional liquid-liquid extraction and solid-phase extraction even SPME and LPME procedures. It involves the partition of analytes between the aqueous and extremely small organic drop and the surface area between the aqueous and organic drop is enhanced dramatically. Thus the extraction time is reduced effectively. Second chapter describes the development of DLLME technique where extraction and derivatization were carried out in one-step. In this work, the derivatizating reagent was added into extraction solvent so that the analytes can be derivatized as the partition of analytes into extraction solvent was carried out. This technique was applied to the analysis of amphetamine and methylenedioxyamphetamine in urine sample from abusers.

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