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C60 之光化學電子自旋研究及 C60 聚合物之合成
Thesis

C60 之光化學電子自旋研究及 C60 聚合物之合成

黃玉蓮
Masters, National Tsing Hua University
1998

Abstract

碳六十電子自旋聚合物 fullereneESRpolymer
I.The fluorescene emission of pyrene was quenched by C60 in various hydrocation solvent, such toluene isodurene etc. The Stern-Volmer plot shows that the fluorescene intensity ratio Io/I is upward, and is non linearly proportional to the fullerene concentration. Electronic absorption measurmes show that pyrene and C60 do not form static complex under the current experimental condition. At a given C60 concentration, increased either solvent polarity or temperature affords diminishment in the ratio . The fluorscene quenching behavior by C70 shows a similar pattern . The data strongly suggest that even at concentration far below saturation, Stern-Volmer fullerene forns aggregates in Organic solvent.II.a stable, broad ESR signal of C60-. anion radical was generated by irradiation of a C60-toluene solution in the presence of organic salt, [(Ph)3P]2N+(Ph)4B-, and 14.3 % methanol. Upon exposure to molecular oxygen, the broad band gradually diminishes and a narrow band of g = 2.0008 and Hpp = 3.32 G grow, which further transforms to another narrow band of g = 2.0026 and Hpp = 1.67 G .The transforation rate found to be negnetive temperature dependent, the higk temperatures and the slower the transfomation .

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