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Synthesis of Hierarchically Porous Structured Bio-Inspired Composites by Diatomites and Freeze Casting
Thesis

Synthesis of Hierarchically Porous Structured Bio-Inspired Composites by Diatomites and Freeze Casting

Lee, Pang Hsuan
Masters, 國立清華大學, 材料科學工程學系
2014

Abstract

矽藻土 冷凍鑄造法 仿生材料 多階層孔洞結構 Diatomite Freeze casting Bio-inspired composites Hierarchical porous structure
Porous composites are widely applied in various fields due to their lightweight, high surface/volume ratio and energy absorbing ability. Natural porous composites, such as bird feathers, beaks and bones, possess lightweight and superior mechanical properties due to their anisotropic, hierarchically porous structure. In this study, we synthesized ultra-lightweight, multifunctional scaffolds mimicking natural porous composites by the freeze casting technique utilizing diatomaceous earth (DE) as raw materials. By controlling the cooling rate, sintering condition and the formation of ice dendritic structures, scaffolds with aligned micro-scaled channels and nano-scaled pores were synthesized. Structural characterization was carried out by SEM and the compositional analysis was identified by XRD. Mechanical properties of DE scaffolds were measured by compressive tests and compared with silica scaffolds. Results showed that two scaffolds had similar ultimate compressive stress and elastic modulus yet DE scaffolds have better toughness and deformability. DE scaffolds were further infiltrated by polymer (PVA) to improve their mechanical properties. The water adsorption, water retention and thermal conductivity of DE scaffolds were also evaluated. The bio-inspired, hierarchically porous scaffolds can be further modified and applied in different fields.

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