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以核磁共振光譜探討臺灣眼鏡蛇心臟毒素V與肝素衍生雙醣的交互作用
Thesis

以核磁共振光譜探討臺灣眼鏡蛇心臟毒素V與肝素衍生雙醣的交互作用

薛光隆
Masters, 國立清華大學, 生物資訊與結構生物研究所
2003

Abstract

心臟毒素 肝素 選擇激發 擴散係數 硫化 cardiotoxin heparin selective excitation DOSY sulfation
In this thesis,we are going to investigate the interaction of the heparinderived disaccharide with the cardiotoxin V (CTX A5). Cardiotoxinswill envenom the target cells and might cause severe necrosis and inflammation,and glycosaminoglycan serve as potential target within the process. The distinct loop regions of CTX A5 differs by two inserts and mutations on the loop I and II make it exhibit much higher affinity to glycosaminoglycans and lipids than other cardiotoxin homologues. From our result of auto-docking and the preliminary x-ray structure suggest the binding of heparin derived disaccharide to CTX A5 is through loop II region and induces protein local conformation change. Compared with the former complex structure CTX A3, CTX A5 complex shows a novel binding site which is consist with the long-chain heparin SPR data. And the binding specificities is proven to depend on the sulfation motif of the disaccharide, thus suggest recognition of CTX A5 to glycosaminoglycans.

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