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單壁奈米碳管量產及其光聲響性質之研究
Thesis

單壁奈米碳管量產及其光聲響性質之研究

曾士豪
Masters, 國立清華大學, 材料科學工程學系
2004

Abstract

單壁奈米碳管 懸浮觸媒法 光聲響 垂直爐管 燃燒 聲波 氧化 奈米碳球 二茂鐵 single wall carbon nanotube floating catalyst method photoacoustic vertical furnace ignition acoustic wave oxidation carbon nanocapsule ferrocene
The high purity fluffy SWNT ball was synthesized through the floating catalyst method in a horizontal tube furnace. Ignition and photoacoustic effects of SWNT ball due to flash exposure were investigated. Acoustic wave accompanied with formation of Fe2SiO4 particles was detected. This phenomenon can be further verified as rapid expansion of surrounding air and carbon oxidation. Ferrocene on fluffy SWNT ignited after flashing, which indicates that the surface temperature of carbon nanotubes after flashing exceeds burning temperature of ferrocene. It also found that the appearance of Fe2SiO4 was related to the existence of iron catalyst. Depending on the catalyst amount in SWNTs, the fluffy ball may ignite or oxidize, according to the response of carbon nanocapsules after flash exposure. The acoustic intensity of fluffy SWNT ball is stronger than that of other carbon materials such as MWNT, carbon fiber, carbon powders etc. Based on the results, it is concluded that the structure transformation of fluffy ball is due to the photoacoustic effect. Moreover, this work established a vertical tube furnace to synthesize the SWNTs with large scale production rate, and a production rate high up to 200 mg/10 min can be achieved. This one dimension SWNT rope can be applied to composite and reinforced materials in the future.

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