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應用臨場照光濕式環境穿透式電子顯微鏡觀測二氧化鈦光催化反應
Thesis

應用臨場照光濕式環境穿透式電子顯微鏡觀測二氧化鈦光催化反應

彭凱麟
Masters, 國立清華大學, 工程與系統科學系
2015

Abstract

電子顯微鏡 二氧化鈦 光催化裂解水 表面非晶化 transmission electron microscopy titanium dioxide light-induced water splitting reaction surface amorphization phenomenon
In this study, we design a fiber-based lightening TEM holder which is compatible with JEOL 2010F and contains a light source illuminating sample along the holder axis that allows sample to be exposed to electron beam and light at the same time. TEM chamber must maintain at ultra-high vacuum environment, so the samples are confined to be in solid state. In order to observe wet samples in TEM, we use the Wet-Cell chips which was designed by our laboratory. This fiber-based lightening TEM holder also can be integrated with Wet Cell chip and provide liquid environment for TEM observation. And it also offers us a chance to in-situ observe the photo-catalytic reaction in real reactional environment. More importantly, we successfully observe the surface amorphization phenomenon in anatase titanium dioxide during UV light irradiation in liquid environment. We also observed the nano-bubbles generation reaction induced by UV light. Use EELS analysis techniques to qualitatively define the oxidation state of titanium in the surface amorphous layer. The valence change is relative to the water splitting reaction mechanism which is induced by UV light through photo-catalysts such as titanium dioxide.

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