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掩飾鄰苯?與單態氧的化學反應
Thesis

掩飾鄰苯?與單態氧的化學反應

高子喬
Masters, National Tsing Hua University
2004

Abstract

單態氧[4+2]反應掩飾鄰苯?光氧化 Singlet oxygenDiels-Alder reactionmasked o-benzoquinonesphotooxygenation
This thesis is concerned with the chemical reaction between MOB and singlet oxygen and deals with the reaction types of MOBs 22a-j and singlet oxygen: Diels-Alder reaction and rearrangement. This thesis is also looking into their possible mechanisms. We have chosen two sensitizers/ solvent systems which are Rose Bengal/ methanol and TPP/ d-chloroform and concluded that d-chloroform preferred the intermediate of biradical to form [4+2] adduct. Furthermore, methanol preferred the intermediate of perepoxide which contains higher energy to form cyclopentenone. However, without such solvent selectivity, 22i and 22j with singlet oxygen produce [4+2] adducts 26i and 26j completely both in d-chloroform and methanol . In the future, after MOB 22e reacts with singlet oxygen, the formation of natural product, Untenone A 24e, can be expected.

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