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樟腦衍生之胺基醇為配位基在不對稱亞□化反應的研究
Thesis

樟腦衍生之胺基醇為配位基在不對稱亞□化反應的研究

鄭丞博
Masters, 國立清華大學, 化學系
2003

Abstract

樟腦 亞□ 催化 camphor sulfoxide catalytic
This thesis dealt with the asymmetric oxidation of sulfide using in situ prepared chiral vanadium complex from tridentate ligands 100-112 with VO(acac)2. The tridentate ligands were synthesized from camphor derived amino alcohols with salicyaldehyde derivates. By using 1.0 eq hydrogen peroxide in portions with 1 mol% vanadium catalyst loading, the best result can be up to 88% ee. In most cases, although the enantioselectivity were moderate, yet the rate of sulfide oxidation was very fast compared with these reported in literature.

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