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磊晶成長氮化銦之光學、電學、熱學性質
Thesis

磊晶成長氮化銦之光學、電學、熱學性質

魏百駿
Masters, National Tsing Hua University
2008

Abstract

氮化銦奈米管柱光譜反光導熱擴散 indium nitridenanotubephotoluminescencenegative photoconductivitythermal diffusivity
In this thesis, we present successful growth and characterization (optical, electrical, and thermal) of InN epitaxial films and nanostructures by molecular beam epitaxy. Temperature-dependent photoluminescence (PL) spectroscopy is used as a tool to study the much controversial optical band gap in degenerate InN. Samples with PL peak on the lower and higher energy side of 0.730 eV demonstrate a normal redshift and anomalous blueshift, respectively, with increasing temperature. This can be explained effectively on the basis of a competition between a conventional red shift from lattice dilation and a blue shift of the electron and hole quasi Fermi-level separation. On the electrical characterization part, we report the first observation of negative photoconductivity behavior in InN thin films. Unlike most conventional (non-degenerate) semiconductors, that show increase in conductivity with illumination, InN shows a regular decrease. The results have been qualitatively modeled on the basis of electronic scattering in the conduction band and transitions in degenerate InN with recombination centers. Finally, a systematic thermal diffusivity (related to thermal conductivity) study in the MBE-grown InN thin films on various substrates with different growth temperatures were carried out. A high thermal diffusivity value of 0.55 cm2/s for a combined 1.7 um thick InN film suggests a lower degree of phonon scattering in our sample with fewer structural defects.

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