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醯亞胺水解?的結晶與X光晶體學分析
Thesis

醯亞胺水解?的結晶與X光晶體學分析

江盛國
Masters, National Tsing Hua University
2002

Abstract

醯亞胺水解? imidase
Imidase also known as dihydropyrimidinase (E.C 3.5.2.2), hydantoinase, dihydropyrimidine hydrase or dihydropyrimidine amidohydrolase, that catalyzes the reversible hydrolysis of 5,6-dihydrouracil to 3-ureidopropionate and many other imides. The degradation of pyrimidine (uracil and thymine) is the only known physiological function of imidase. In vitro data indicate that imidase has a broad substrate specificity and prefer xenobiotics over natural substrates. Substrate specificity, metal content and amino-acid sequence all differ significantly between bacterial and mannalian imide-hydrolyzing enzymes. In our study, a thermophilic imidase were purified from pig liver and Agrobacterium radiobacter and crystallized. In pig liver imidase, two kinds of imidase crystals were grown by the hanging-drop vapor-diffusion method using polyethylene glycol MME 5000 and 2-propanol as precipitants. One belongs to the triclinic P1 space group,with unit-cell parameters a = 96.35A, b = 96.87A, c = 154.87A, □ = 82.10o, □ = 72.54o, □ = 77.19o, and the other belongs to the orthorhombic C2221 space group, with unit-cell parameters a = 113.92A, b =157.22A, c =156.21A. In the Agrobacterium radiobacter imidase (A. radio.- D-hydantoinase), two kinds of imidase crystals were grown by the hanging-drop vapor-diffusion method using ammonium sulfate as precipitant. One belongs to cubic F23 (or rhombohedral R3) space group, with unit-cell parameters a = b = c =179.73A (a = b = 127.09A, c = 311.29A, □ = 120o), and the other belongs to tetragonal I4 space group, with unit-cell parameters a = b =129.39A, c = 173.31A.

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