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鈀錯合物催化丙二烯,醯氯化合物,有機錫試劑之三組成反應
Thesis

鈀錯合物催化丙二烯,醯氯化合物,有機錫試劑之三組成反應

蔡麗菁
Masters, 國立清華大學, 化學系
1999

Abstract

鈀金屬 丙二烯 醯氯化合物 三組成反應 palladium allene acid chloride three-component coupling reaction
Acyl chlorides R1COCl, allenes R2R3CCCH2 and organotin reagents Bu3SnR4 undergo three-component coupling reaction in toluene in the presence of Pd(dba)2 to give functionally substituted a, b unsaturated ketones R2R3C=C(COR1)CH2R4. Based on known palladium-allene and -allyl chemistry, we propose a mechanism to account for this palladium-catalyzed three-component coupling reactions.

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