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電漿噴塗法成長具奈米結構之固態氧化物燃料電池陽極薄膜Ni/YSZ 之結構與電性分析
Thesis

電漿噴塗法成長具奈米結構之固態氧化物燃料電池陽極薄膜Ni/YSZ 之結構與電性分析

楊燿瑜
Masters, 國立清華大學, 工程與系統科學系
2004

Abstract

固態氧化物燃料電池 陽極 活化極化損失 奈米顆粒 三相態 孔隙率 SOFC Anode Activation polarization loss Nano particle Three phase boundary porosity
In this research, we fabricated the nano-particle structure of solid oxide fuel cell (SOFC) anode film by thermal plasma spray coating, which produced a homogeneous layer of NiO/YSZ mixture coated on the YSZ substrate. Then, reduce the sample of NiO/YSZ to Ni/YSZ by mixture gas (7 % H2 + 93 % Ar) in high temperature (800℃). After reduction, the particle size of film of the SOFC anode is about 50 nm. In our sample, we estimated the number of three phase boundary (TPB) is about 3~4 orders of magnitude better than micro scale particles. The result can obviously increase the electrochemical reaction area in SOFC anode. The single layer of anode is highly conductive with 1000 S/cm in room temperature. We observed the morphology and structure of SOFC anode by X-ray powder diffraction (XRD) 、scanning electron microscopy (SEM) 、 atomic force microscopy (AFM) and Brunauer-Emmett-Teller (BET). These tools can help us observed the characteristic of nano-particle in SOFC anode.

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