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Chemically induced dynamic nuclear polarization in systems containing large hyperfine coupling constants
Journal article

Chemically induced dynamic nuclear polarization in systems containing large hyperfine coupling constants

Heinz D. Roth, Richard S. Hutton, Kuo-Chu Hwang, Nicholas J. Turro and Kevin M. Welsh
Journal of Physical Chemistry, Vol.93(15), pp.5697-5701
1989

Abstract

Nuclear spin polarization effects induced in radical pairs with one or more strong ( 13 C) hyperfine coupling constants have been evaluated. The pairs were generated by photoinduced α-cleavage or hydrogen abstraction reactions of carbonyl compounds. Several examples illustrate how changes in the magnetic field strength (H 0 ) and the g-factor difference (Δ g ) affect the general appearance of the resulting CIDNP multiplets. The results bear out an earlier caveat concerning the qualitative interpretation of CIDNP effects observed for multiplets. © 1989 American Chemical Society.

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