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Combined Gadolinium and Boron Neutron Capture Therapies for Eradication of Head-and-Neck Tumor Using Gd10B6 Nanoparticles under MRI/CT Image Guidance
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Combined Gadolinium and Boron Neutron Capture Therapies for Eradication of Head-and-Neck Tumor Using Gd10B6 Nanoparticles under MRI/CT Image Guidance

Munusamy Shanmugam, Naresh Kuthala, Xiangyi Kong, Chi-Shiun ChiangKuo Chu Hwang
JACS Au
2023

摘要

boron neutron capture therapy dual contrast agent gadolinium neutron capture therapy hypoxia recurrent head and neck cancer tumor biomarkers Analytical Chemistry Chemistry (miscellaneous) Physical and Theoretical Chemistry Organic Chemistry
Eradication of head-and-neck (H&N) tumors is very difficult and challenging because of the characteristic feature of frequent recurrence and the difficulty in killing cancer stem cells. Neutron capture therapy (NCT) is emerging as a noninvasive potential modality for treatments of various types of tumors. Herein, we report that 98.5% <sup>10</sup> B-enriched anti-EGFR-Gd <sup>10</sup> B <sub>6</sub> nanoparticles can not only deliver large doses of 158 μg <sup>10</sup> B/g tumor tissues as well as 56.8 μg <sup>157</sup> Gd/g tumor tissues with a very high tumor-to-blood (T/B) <sup>10</sup> B ratio of 4.18, but also exert very effective CT/MRI image-guided combined GdBNCT effects on killing cancer stem cells and eradication of recurrent head-and-neck (H&N) tumors. This leads to a long average half-lifespan of 81 days for H&N tumor-bearing mice, which is a record-making result, and surpasses the best result reported in the literature using combined radiotherapy and T cell-mediated immunotherapy (70 d).

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https://doi.org/10.1021/jacsau.3c00250檢視
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