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Crystal-encapsulation-induced band-structure change in single-walled carbon nanotubes: Photoluminescence and Raman spectra
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Crystal-encapsulation-induced band-structure change in single-walled carbon nanotubes: Photoluminescence and Raman spectra

Lain-Jong Li, Tsung-Wu Lin, J. Doig, I.B. Mortimer, J.G. Wiltshire, R.A. Taylor, J. Sloan, M.L.H. GreenR.J. Nicholas
Physical Review B - Condensed Matter and Materials Physics, 卷.74(24), 245418
2006

摘要

Electronic Optical and Magnetic Materials Condensed Matter Physics
We report studies of the modification of the band structure of single-walled carbon nanotubes through encapsulation of the inorganic material manganese ditelluride (Mn Te2). Using photoluminescence excitation mapping we show that this leads to a global reduction of their first and second band gap energies by a similar percentage (up to 3.8%). We interpret this as due to the additional screening which causes a change in the internal dielectric constant and a possible lowering of the carbon-carbon transfer integrals. The shifts increase with increasing tube diameter due to the increased quantity of filled materials. © 2006 The American Physical Society.

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