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Diameter-selective encapsulation of metallocenes in single-walled carbon nanotubes
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Diameter-selective encapsulation of metallocenes in single-walled carbon nanotubes

Lain-Jong Li, A.N. Khlobystov, J.G. Wiltshire, G.A.D. BriggsR.J. Nicholas
Nature Materials, 卷.4(6), 頁碼.481-485
2005
PMID: 15908958

摘要

Chemistry (all) Materials Science (all) Condensed Matter Physics Mechanics of Materials Mechanical Engineering
The diameter selective encapsulation of two metallocene compounds bis(cyclopentadienyl) cobalt and bis(ethylcyclopentadienyl) was analyzed in single-walled carbon nanotubes. Electron transfer from the cobalt ions to the nanotubes was directly observed through a change in the charge state of the encapsulated molecule. Two very strong absorption bands for CoCp 2 at 5.277 eV and 4.788 eV were assigned to the metal-to-ligand and ligand-to-metal charge transfer transitions. It was observed that the absorption of CoCp 2 in a relatively wide nanotube was only slightly exothermic.

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