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Different roles of trifluoromethanesulfonyl chloride in the construction of heterocycles fused with β-lactams
Journal article   Peer reviewed

Different roles of trifluoromethanesulfonyl chloride in the construction of heterocycles fused with β-lactams

Jih Ru Hwu, Shahram Hakimelahi, Kuang-Lieh Lu and Shwu-Chen Tsay
Tetrahedron, Vol.55(26), pp.8039-8044
25/06/1999

Abstract

The cis-configurated tricyclic O 3 -isooxacepham 5 and bicyclic isopenam 11 were synthesized. The key step for the preparation of 5 involves chlorination of the corresponding carbanion of 3 with CF 3 SO 2 Cl followed by an internal alkylation. The biologically active isopenam 11 was synthesized from thio-S-ester 6 via intermediate 9. The key step involves chlorination of the thiol moiety in monocyclic β-lactam 7 by CF 3 SO 2 Cl followed by an internal cyclization.

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