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Electrocatalytic Reduction of Carbon Dioxide with a Well-Defined PN3-Ru Pincer Complex
期刊文章

Electrocatalytic Reduction of Carbon Dioxide with a Well-Defined PN3-Ru Pincer Complex

Shixiong Min, Shahid Rasul, Huaifeng Li, David C. Grills, Kazuhiro Takanabe, Lain-Jong LiKuo-Wei Huang
ChemPlusChem, 卷.81(2), 頁碼.166-171
02/2016

摘要

electrocatalysts electrochemistry N,P ligands redox ruthenium Chemistry (all)
A well-defined PN 3 -Ru pincer complex (5) bearing a redox-active bipyridine ligand with an aminophosphine arm has been established as an effective and stable molecular electrocatalyst for CO 2 reduction to CO and HCOOH with negligible formation of H 2 in a H 2 O/MeCN mixture. Done in a pince: A PN 3 -Ru pincer complex (see figure) has been found to show high activity and stability as a molecular electrocatalyst for CO 2 reduction to CO and HCOOH in MeCN/H 2 O.

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