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Flexo-phototronic effect in centro-symmetric BiVO4 epitaxial films
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Flexo-phototronic effect in centro-symmetric BiVO4 epitaxial films

Pao-Wen Shao, Meng-Chin Lin, Qian Zhuang, Jiawei Huang, Shi Liu, Hsiao-Wen Chen, Hsiang-Lin Liu, Yu-Jung Lu, Yung-Jung Hsu, Jyh-Ming Wu, …
Applied Catalysis B: Environmental, 卷.312, 121367
09/2022

摘要

Centro-symmetry Domain wall Flexo-phototronic Flexoelectricity Strain gradient Catalysis Environmental Science (all) Process Chemistry and Technology
With exciting functionality, topological defects in ferroic system have attracted significant attention. Under proper design, the emergence of polar domain walls in non-polar ferroelastics enables a flexo-phototronic effect. In this study, we revealed ferroelastic twin texture with localized flexoelectric effect in centrosymmetric epitaxial BiVO 4 film. Supported by photodeposition and localized photocurrent analysis, we found the flexoelectric effect confined at domain wall area facilitates the photocarrier transport and the flexo-phototronic mechanism was further supported by dye-degradation and generation of reactive radicals. This work not only provides new insights into the introduction of flexo-phototronic effects in non-polar materials, but also sheds light on the use of material inhomogeneity for acquiring multifunctionality.

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