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Formation of nanowire striations driven by marangoni instability in spin-cast polymer thin films
Journal article   Peer reviewed

Formation of nanowire striations driven by marangoni instability in spin-cast polymer thin films

Shih-Yuan Lu, Kuen-Hua Wu and Yen-Yi Chen
Langmuir, Vol.23(20), pp.10069-10073
25/09/2007

Abstract

Parallel striations made of silver nanowires were formed through the Marangoni instability induced during spin casting of poly (2-vinyl pyridine)/silver nano wire/chloroform solutions. The striation patterns of the silver nanowires resembled those obtained from spin casting of the corresponding neat polymer solutions, indicating essentially the same driving mechanism (i.e., the Marangoni instability). The silver nanowires were found to concentrate in the valleys of the striation pattern to balance the nonuniform surface tension distribution in the polymer thin film. The resulting nanowire striation patterns were found to depend on polymer concentration, rotational speed, and nanowire loading. Interestingly, this nanowire striation phenomenon was found to be independent of the substrate characteristics, hydrophobic or hydrophilic. © 2007 American Chemical Society.

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