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Gamma-ray engineered surface defects on zinc oxide nanorods towards enhanced NO2 gas sensing performance at room temperature
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Gamma-ray engineered surface defects on zinc oxide nanorods towards enhanced NO2 gas sensing performance at room temperature

Aswin kumar Anbalagan, Shivam Gupta, Rishi Ranjan Kumar, Anupam Ruturaj Tripathy, Mayur Chaudhary, Shu-Chih Haw, Thangapandian Murugesan, Heh-Nan Lin, Yu-Lun Chueh, Nyan-Hwa Tai, …
Sensors and Actuators B: Chemical, 卷.369, 132255
10/2022

摘要

Gamma-ray irradiation Gas sensor Hydrothermal method ZnO Electronic Optical and Magnetic Materials Instrumentation Condensed Matter Physics Surfaces Coatings and Films Metals and Alloys Electrical and Electronic Engineering Materials Chemistry
Gamma-ray irradiation is a fast and efficient technique that can constructively create various defects in a controlled manner to tune materials’ functionality. In this work, zinc oxide nanorods are hydrothermally grown over flexible polyethylene terephthalate paper substrate and then irradiated with 60 Co gamma-ray source to create various defects for possible enrichment towards NO 2 gas sensing. The sensors irradiated with gamma-ray show enhanced NO 2 responses of 120%, 160%, and 185% for 500 ppb concentration at the irradiation doses of 1.5 kGy, 4.5 kGy, and 6 kGy, respectively, as compared to the pristine sensor response of 80%. Maximum response of 312% is achieved at the irradiation dose of 6 kGy for 1500 ppb of NO 2 . Overall, this study confirms that the enhanced oxygen vacancies, defect concentration, and increased grain boundaries, caused by gamma-ray irradiation can eventually achieve more than two times better efficiency towards NO 2 detection at room temperature (25 ℃) on a flexible based NO 2 sensor.

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