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Hysteresis-Free Contact Doping for High-Performance Two-Dimensional Electronics
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Hysteresis-Free Contact Doping for High-Performance Two-Dimensional Electronics

柏勳 何, Jun-Ru Chang, Chun-Hsiang Chen, Cheng-Hung Hou, Chun-Hao Chiang, Min-Chuan Shih, Hung-Chang Hsu, Wen-Hao Chang, Jing-Jong Shyue, Ya-Ping Chiu, …
ACS Nano, 卷.17(3), 頁碼.2653-2660
30/01/2023

摘要

two-dimensional materials;contact doping;n-type doping;hysteresis;transistors;contact resistance;scanning tunneling microscopy

Contact doping is considered crucial for reducing the contact resistance of two-dimensional (2D) transistors. However, a process for achieving robust contact doping for 2D electronics is lacking. Here, we developed a two-step doping method for effectively doping 2D materials through a defect-repairing process. The method achieves strong and hysteresis-free doping and is suitable for use with the most widely used transition-metal dichalcogenides. Through our method, we achieved a record-high sheet conductance (0.16 mS·sq–1 without gating) of monolayer MoS2 and a high mobility and carrier concentration (4.1 × 1013 cm–2). We employed our robust method for the successful contact doping of a monolayer MoS2 Au-contact device, obtaining a contact resistance as low as 1.2 kΩ·μm. Our method represents an effective means of fabricating high-performance 2D transistors.

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