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Nano-scale mechanical characteristics of epitaxial stabilization ZrTiN/NbN superlattice coatings
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Nano-scale mechanical characteristics of epitaxial stabilization ZrTiN/NbN superlattice coatings

Tsai-Ni Ku, Sheng-Yu Hsu, Yuan-Tai Lai, Shou-Yi Chang, Su-Yueh TsaiJenq-Gong Duh
Surface and Coatings Technology, 卷.453, 129123
01/2023

摘要

Epitaxial stabilization Hard-yet-tough coatings Nano-scale tribological properties Superlattices Transition metal nitride Chemistry (all) Condensed Matter Physics Surfaces and Interfaces Surfaces Coatings and Films Materials Chemistry
Protective hard thin films are necessary in industrial engineering under extreme condition. In that regard, superlattices with epitaxial stabilization have shown to be a potential approach. The ZrTiN/NbN system was chosen due to the similar lattice parameter and crystal structure. The phase transition from c-NbN to h-NbN was presented while NbN sub-layer was relatively thick in the superlattices, owing to higher VEC (valence electron concentration) of NbN. HRTEM images confirmed that h-NBN led to the loss of epitaxial growth, and thus the coatings demonstrated polycrystalline structure. The superlattices showed no cracks after indentation, possessing stronger crack resistance than ZrTiN (K c = 3.22 MPa √ m) and NbN (K c = 2.70 MPa √ m) monolayers. A 3-scan procedure was conducted and multilayers exhibited the staircase-like curve during scratching. The wear volume of multilayers was significantly lower than monolithic films, however, the existence of h-NbN would deteriorate the wear resistance and elastic recovery of the coatings. It can be concluded that epitaxial ZrTiN/c-NbN superlattices exhibited not only favorable mechanical performance but also excellent tribological behavior.

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