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Nonlinear Stern-Volmer fluorescence quenching of pyrene by C60/70
Journal article

Nonlinear Stern-Volmer fluorescence quenching of pyrene by C60/70

Yu Lien Hwang and Kuo Chu Hwang
Fullerene Science and Technology, Vol.7(3), pp.437-454
1999

Abstract

The Stern-Volmer plot of fluorescence quenching of pyrene by C <sub>60</sub> (or C <sub>70</sub> ) is upward, and non linearly proportional to the fullerene concentration. Electronic absorption measurements show that pyrene and C <sub>60</sub> do not form static complexes under the experimental condition. A novel 'inner filter effect' model is proposed to rationalize the observed non linear upward Stern Volmer behavior. At a given C <sub>60</sub> concentration, increasing either solvent polarity or temperature (T>280 K) causes diminishment in the I <sub>0</sub> /I ratio. The data strongly suggest that even at concentrations far below saturation, fullerenes form aggregates in organic solvents.

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