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Numerical analysis of transport and retardation for cesium in crushed granite using multi-stage advection-dispersion column experiments
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Numerical analysis of transport and retardation for cesium in crushed granite using multi-stage advection-dispersion column experiments

Chuan-Pin Lee, Ming-Chee Wu, Shih-Chin Tsai, Ching-Yuan Liu, Tsuey-Lin Tsai, Chun-Hua Pan 和 Mon-Shieh Yang
Journal of radioanalytical and nuclear chemistry, 卷.304(1), 頁碼.377-386
01/04/2015
Web of Science ID: WOS:000351755200057

摘要

Chemistry Chemistry, Analytical Chemistry, Inorganic & Nuclear Nuclear Science & Technology Physical Sciences Science & Technology Technology
In this study, a systematic analysis of cesium through crushed granite (0.297-0.840 mm) was constructed where synthetic groundwater and seawater were employed as the liquid phase. To build such models, multi-stage advection-dispersion column tests were conducted in order to determine the major transport processes and the calibration/validation of the hypothesized reactive transport models. The experimental breakthrough curves (BTCs) for HTO and Cs were both matched with their corresponding numerical BTCs by adjusting reaction and transport parameters such as forward or backward reaction rate constants (k(f) or k(b)), dispersivity (alpha), and porosity(theta).

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