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Optimization of alkali fusion process for determination of I-129 in solidified radwastes by neutron activation
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Optimization of alkali fusion process for determination of I-129 in solidified radwastes by neutron activation

Jiunn-Hsing Chao, Chun-Yu Chuang, Wei-Chun Chou, Chun-Liang Kuo, Feng-Chih ChangAn-Chung Chiang
Applied Radiation and Isotopes, 卷.176, 109762
10/2021

摘要

129I Alkali fusion Neutron activation analysis Radwaste Radiation
This study determines the optimum temperature for the alkali fusion process used to effectively separate iodine from solidified radwaste attaining low-level 129 I by neutron activation. The alkali fusion temperature was adjusted to 120, 200, and 400 °C to approach the optimum conditions associated with a good statistical distribution of the measured 129 I data and high chemical recovery yield. Statistical analysis revealed that the optimum temperature of the alkali fusion process was 200 °C, displaying good central tendency and low variance of the measured 129 I data, and the respective chemical recovery yields were higher than other temperatures. The optimum fusion condition provides more reliable scaling factors ( 129 I/ 137 Cs) of radwaste.

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1 檢視次數

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