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Proximity induced charge density wave in a graphene/1T-TaS2 heterostructure
期刊文章

Proximity induced charge density wave in a graphene/1T-TaS2 heterostructure

N. Tilak, M. Altvater, S.-H. Hung, C.-J. Won, G. Li, T. Kaleem, S.-W. Cheong, C.-H. Chung, H.-T. Jeng 和 E.Y. Andrei
Nature Communications, 卷.15(1)
2024
Web of Science ID: WOS:001335565900009

摘要

graphene coexistence numerical model reduction spectroscopy superconductivity theoretical study ab initio calculation Article charge density controlled study density functional theory Fourier transform hexagonal crystal high temperature magnetism mathematical model phonon scanning tunneling microscopy superconductivity topography adult article dispersion electron spectroscopy
The proximity-effect, whereby materials in contact appropriate each other’s electronic-properties, is widely used to induce correlated states, such as superconductivity or magnetism, at heterostructure interfaces. Thus far however, demonstrating the existence of proximity-induced charge-density-waves (PI-CDW) proved challenging. This is due to competing effects, such as screening or co-tunneling into the parent material, that obscured its presence. Here we report the observation of a PI-CDW in a graphene layer contacted by a 1T-TaS2 substrate. Using scanning tunneling microscopy (STM) and spectroscopy (STS) together with theoretical-modeling, we show that the coexistence of a CDW with a Mott–gap in 1T-TaS2 coupled with the Dirac-dispersion of electrons in graphene, makes it possible to unambiguously demonstrate the PI-CDW by ruling out alternative interpretations. Furthermore, we find that the PI-CDW is accompanied by a reduction of the Mott gap in 1T-TaS2 and show that the mechanism underlying the PI-CDW is well-described by short-range exchange-interactions that are distinctly different from previously observed proximity effects. © The Author(s) 2024.

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https://www.scopus.com/inward/record.uri?eid=2-s2.0-85203984654&doi=10.1038%2fs41467-024-51608-y&partnerID=40&md5=6a2bb1046cbc8788d93b6d36b2913ee3檢視
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