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Pt- and Au-catalyzed oxidative cyclization of 2-ethenyl-1-(prop-2′- yn-1′-ol)benzenes to naphthyl aldehydes and ketones: Catalytic oxidation of metal-alkylidene intermediates using H2O and H2O 2
Journal article   Peer reviewed

Pt- and Au-catalyzed oxidative cyclization of 2-ethenyl-1-(prop-2′- yn-1′-ol)benzenes to naphthyl aldehydes and ketones: Catalytic oxidation of metal-alkylidene intermediates using H2O and H2O 2

Bhanu Pratap Taduri, Shariar Md. Abu Sohel, Hsin-Mei Cheng, Guan-You Lin and Rai-Shung Liu
Chemical Communications, (24), pp.2530-2532
2007

Abstract

2-Ethenyl-1-(prop-2′-yn-1′-ol)benzenes was cyclized through catalytic oxidation with PtCl 2 /CO/H 2 O and PEt 3 AuCl/H 2 O 2 ; the metal-naphthylidene intermediates were identified and oxygenated with water and H 2 O 2 , respectively; for the efficiency of cyclization, the Au catalytic system is superior to that of the PtCl 2 -catalysis because of its compatibility toward diverse alcohol substrates including both internal alkynes and terminal alkynes. © The Royal Society of Chemistry.

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