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Revealing the flexoelectricity in the mixed-phase regions of epitaxial BiFeO3 thin films
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Revealing the flexoelectricity in the mixed-phase regions of epitaxial BiFeO3 thin films

Cheng-En Cheng, Heng-Jui Liu, Franco Dinelli, Yi-Chun Chen, Chen-Shiung Chang, Forest Shih-Sen ChienYing-Hao Chu
Scientific Reports, 卷.5, 8091
01/2015

摘要

Multidisciplinary
Understanding the elastic response on the nanoscale phase boundaries of multiferroics is an essential issue in order to explain their exotic behaviour. Mixed-phase BiFeO 3 films, epitaxially grown on LaAlO 3 (001) substrates, have been investigated by means of scanning probe microscopy to characterize the elastic and piezoelectric responses in the mixed-phase region of rhombohedral-like monoclinic (M I ) and tilted tetragonal-like monoclinic (M II,tilt ) phases. Ultrasonic force microscopy reveal that the regions with low/high stiffness values topologically coincide with the M I /M II,tilt phases. X-ray diffraction strain analysis confirms that the M I phase is more compliant than the M II,tilt one. Significantly, the correlation between elastic modulation and piezoresponse across the mixed-phase regions manifests that the flexoelectric effect results in the enhancement of the piezoresponse at the phase boundaries and in the M I regions. This accounts for the giant electromechanical effect in strained mixed-phase BiFeO 3 films.

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https://doi.org/10.1038/srep08091檢視
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