Logo image
Shift of charge inversion point of a trivalent ion solution in a nanofluidic channel
期刊文章   開放取用(OA)

Shift of charge inversion point of a trivalent ion solution in a nanofluidic channel

Kyojiro MorikawaTakehiko Tsukahara
Colloids and Interface Science Communications, 卷.50, 頁.100646
09/2022

摘要

Charge inversion;Nanochannel;Nanofluidics;Streaming current;Zeta potential Biotechnology Physical and Theoretical Chemistry Surfaces Coatings and Films Colloid and Surface Chemistry Materials Chemistry

Understanding the surface properties and related liquid properties in 10 2 nm spaces (extended nanospaces) is critical for future device engineering. To this end, we used trivalent ions to investigate the charge inversion phenomenon in extended nanospaces. The charge inversion points in bulk didn't substantially differ between a La(NO 3 ) 3 solution and a Lu(NO 3 ) 3 solution. However, the charge inversion point of a La(NO 3 ) 3 solution in extended nanochannels shifted toward the higher-concentration region. The conductivity measurement results suggested a negatively charged surface in the extended nanospaces in the La(NO 3 ) 3 solution, consistent with the zeta-potential results. In addition, a much increase in the 1/T 1 of the La(NO 3 ) 3 solution was shown compared with that of the bulk. We report a new finding that different trivalent ions exhibit different adsorption properties but only in extended nanospaces, not in bulk. We expect our results to contribute to the basic science to understand the liquid properties in nanospaces.

檔案與連結 (1)

url
https://doi.org/10.1016/j.colcom.2022.100646檢視
已出版(紀錄版本) 開放

相關連結

指標

1 檢視次數

詳細資料

Logo image