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Spatially and temporally-resolved tryptophan fluorescence thermometry for monitoring the photothermal processes of gold nanorod suspensions
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Spatially and temporally-resolved tryptophan fluorescence thermometry for monitoring the photothermal processes of gold nanorod suspensions

Chia-Te Lin, Kuan-Jen Chen, Ke-Chia TsengLi-Kang Chu
Sensors and Actuators, B: Chemical
2017

摘要

Confocal fluorescent thermometer;Gold nanorods;Thermal infrared imaging;Tryptophan Electronic Optical and Magnetic Materials Instrumentation Condensed Matter Physics Surfaces Coatings and Films Metals and Alloys Materials Chemistry Electrical and Electronic Engineering

We constructed a confocal fluorescent thermometer to monitor the spatial and temporal temperature evolutions of gold nanorod suspensions upon continuous-wave infrared excitation. Tryptophan served as the fluorophore due to its superior temperature dependent fluorescence intensity, ca. -2%°C -1 . We provided sufficient spatial resolution of 50μm and temperature sensitivity of 0.3°C. Coupled with an infrared thermocamera, we were able to obtain simultaneously the temperature evolutions in the bulk solution and on the container surface. Employment of this noncontact and optical approach allows investigation of the thermal distribution in a minute volume, less than 1mm 3 , without the additional perturbative factors of the mechanical thermometers, e.g., the thermal conductivity and volume of the sensor.

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