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Strain induced metal-insulator transition of magnetic SrRuO3 single layer in SrRuO3/SrTiO3 superlattice
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Strain induced metal-insulator transition of magnetic SrRuO3 single layer in SrRuO3/SrTiO3 superlattice

Angus Huang, Sheng-Hsiung HungHorng-Tay Jeng
Applied Sciences (Switzerland), 卷.8(11), 2151
11/2018

摘要

2D Half-metal Magnetism Metal-insulator transition Superlattice Materials Science (all) Instrumentation Engineering (all) Process Chemistry and Technology Computer Science Applications Fluid Flow and Transfer Processes
Ferromagnetic phase in a two-dimensional system plays an important role not only in applications but also in studies of phase transition theory. Among numerous ferromagnetic materials, SrRuO 3 is famous for its half-metallicity, itinerant ferromagnetism and non-Fermi liquid metalicity. Single layer SrRuO 3 in SrRuO 3 /SrTiO 3 (SRO/STO) superlattice has been predicted as a two-dimensional half-metallic ferromagnetic system based on density functional theory (DFT). However, experiments show that metal-insulator transition associated with ferro-antiferromagnetism (FM-AFM) transition occurs when the thickness of SRO is less than 4 u.c. Combining DFT calculations with Monte Carlo simulations, we demonstrate in this work that the bulk ferromagnetic metallicity can be realized in single layer SRO in SRO/STO superlattice by manipulating the strain effect to trigger the metal-insulator transition, achieving two-dimensional (2D) half-metallic SRO thin film beyond the experimental observation of AFM insulator.Our results pave a new route to fulfill the ultrathin spin-polarized-2D electron gas (SP-2DEG).

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https://doi.org/10.3390/app8112151檢視
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