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Symmetric synergy of hybrid CoS2-WS2 electrocatalysts for the hydrogen evolution reaction
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Symmetric synergy of hybrid CoS2-WS2 electrocatalysts for the hydrogen evolution reaction

Xiaofeng Zhou, Xiulin Yang, Henan Li, Mohamed Nejib Hedhili, Kuo-Wei Huang, Lain-Jong LiWenjing Zhang
Journal of Materials Chemistry A, 卷.5(30), 頁碼.15552-15558
2017

摘要

Chemistry (all) Renewable Energy Sustainability and the Environment Materials Science (all)
A highly active and stable hybrid electrocatalyst 3D hierarchical CoS 2 nanosheets incorporated with WS 2 (CoS 2 @WS 2 ) has been developed via a one-step sulfurization method for the first time, where the contents of WS 2 can be adjusted easily. We first prove that the addition of small amounts of WS 2 enhances the hydrogen evolution reaction (HER) performance of CoS 2 , and vice versa. In other words, we validated the symmetric synergy for the HER between the Co- and W-based sulfide hybrid catalysts. In addition, we confirmed that the formation of nanointerfaces of Co-S-W between CoS 2 and WS 2 was responsible for the excellent HER activity (an overpotential of -97.2 mV at -10 mA cm -2 , a small Tafel slope of 66.0 mV dec -1 , and prominent electrochemical stability) of the hybrid electrocatalyst CoS 2 @WS 2 .

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