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Synthesis of the extended phenacene molecules, [10]phenacene and [11]phenacene, and their performance in a field-effect transistor
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Synthesis of the extended phenacene molecules, [10]phenacene and [11]phenacene, and their performance in a field-effect transistor

Hideki Okamoto, Shino Hamao, Ritsuko Eguchi, Hidenori Goto, Yasuhiro Takabayashi, Paul Yu-Hsiang Yen, Luo Uei Liang, Chia-Wei Chou, Germar Hoffmann, Shin Gohda, …
Scientific Reports, 卷.9(1), 4009
12/2019
PMID: 30850618

摘要

Multidisciplinary
The [10]phenacene and [11]phenacene molecules have been synthesized using a simple repetition of Wittig reactions followed by photocyclization. Sufficient amounts of [10]phenacene and [11]phenacene were obtained, and thin-film FETs using these molecules have been fabricated with SiO <sub>2</sub> and ionic liquid gate dielectrics. These FETs operated in p-channel. The averaged measurements of field-effect mobility, <μ>, were 3.1(7) × 10 <sup>−2</sup> and 1.11(4) × 10 <sup>−1</sup> cm <sup>2</sup> V <sup>−1</sup> s <sup>−1</sup> , respectively, for [10]phenacene and [11]phenacene thin-film FETs with SiO <sub>2</sub> gate dielectrics. Furthermore, [10]phenacene and [11]phenacene thin-film electric-double-layer (EDL) FETs with ionic liquid showed low-voltage p-channel FET properties, with <μ> values of 3(1) and 1(1) cm <sup>2</sup> V <sup>−1</sup> s <sup>−1</sup> , respectively. This study also discusses the future utility of the extremely extended π-network molecules [10]phenacene and [11]phenacene as the active layer of FET devices, based on the experimental results obtained.

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https://doi.org/10.1038/s41598-019-39899-4檢視
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