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Thioether-ligated iron(ii) and iron(iii)-hydroperoxo/alkylperoxo complexes with an H-bond donor in the second coordination sphere
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Thioether-ligated iron(ii) and iron(iii)-hydroperoxo/alkylperoxo complexes with an H-bond donor in the second coordination sphere

Leland R. Widger, Yunbo Jiang, Alison C. McQuilken, Tzuhsiung Yang, Maxime A. Siegler, Hirotoshi Matsumura, Pierre Moënne-Loccoz, Devesh Kumar, Sam P. De VisserDavid P. Goldberg
Dalton Transactions, 卷.43(20), 頁碼.7522-7532
05/2014
PMID: 24705907

摘要

Inorganic Chemistry
The non-heme iron complexes, [Fe II (N3PySR)(CH 3 CN)](BF 4 ) 2 (1) and [Fe II (N3Py amide SR)](BF 4 ) 2 (2), afford rare examples of metastable Fe(iii)-OOH and Fe(iii)-OOtBu complexes containing equatorial thioether ligands and a single H-bond donor in the second coordination sphere. These peroxo complexes were characterized by a range of spectroscopic methods and density functional theory studies. The influence of a thioether ligand and of one H-bond donor on the stability and spectroscopic properties of these complexes was investigated. This journal is © the Partner Organisations 2014.

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