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Triflic acid-promoted formylation of ceramide in dimethyl foramide
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Triflic acid-promoted formylation of ceramide in dimethyl foramide

Liwu Chiang, Sider Pan, Jemmau LoChungshan Yu
Chinese Journal of Chemistry Chinese Journal of Chemistry, 卷.27, 頁碼.2296-2299
2009

摘要

ceramide;rearrangement;oxazole
The protected ceramide: N-((2S,3S,4R)-3,4-bis(benzyloxy)-1-hydroxyoctadecan-2-yl)tetracosanamide, was attempted to introduce a triflate as a leaving group followed by a nucleophilic substitution with azido group in one-pot manner. Unexpectedly, the oxazole ring formed via a thermodynamically favored intramolecular cyclization was opened to generate the original ceramide by triflic acid. In addition, the residual acid promoted a formylation of the primary hydroxy group in DMF.

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