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Ultrafast Giant Photostriction of Epitaxial Strontium Iridate Film with Superior Endurance
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Ultrafast Giant Photostriction of Epitaxial Strontium Iridate Film with Superior Endurance

Jan-Chi Yang, Yi-De Liou, Wen-Yen Tzeng, Heng-Jui Liu, Yao-Wen Chang, Ping-Hua Xiang, Zaoli Zhang, Chun-Gang Duan, Chih-Wei Luo, Yi-Chun Chen, …
Nano Letters, 卷.18(12), 頁碼.7742-7748
12/2018
PMID: 30407834

摘要

complex oxide giant photostriction with superior endurance Raman scattering SrIrO 3 time-resolved transient microscopy ultrafast orientation-resolved pump-probe spectroscopy Bioengineering Chemistry (all) Materials Science (all) Condensed Matter Physics Mechanical Engineering
Photostriction, optical stimulus driven mechanical deformation in materials, provides a solution toward next-generation technology. Here, the giant photostriction (∼2% change of lattice) of epitaxial strontium iridate (SrIrO 3 ) films under illumination at room temperature is revealed via power-dependent Raman scattering, which is significantly larger as compared to conventional inorganic materials. The time scale and mechanism of this giant photostriction in SrIrO 3 are further studied through time-resolved transient reflectivity measurements. The main mechanism is determined to be the electron-phonon coupling. In addition, we find that such an exotic behavior happens within few picoseconds and remains up to 10 7 cyclic on/off operations. The observation of giant photostriction in SrIrO 3 films with superior endurance promises the advance of shape responsive solids that are sensitive to environmental stimuli, which could be widely utilized for multifunctional optoelectronics and optomechanical devices.

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