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Visible Light Copper Photoredox-Catalyzed Aerobic Oxidative Coupling of Phenols and Terminal Alkynes: Regioselective Synthesis of Functionalized Ketones via CC Triple Bond Cleavage
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Visible Light Copper Photoredox-Catalyzed Aerobic Oxidative Coupling of Phenols and Terminal Alkynes: Regioselective Synthesis of Functionalized Ketones via CC Triple Bond Cleavage

Arunachalam Sagadevan, Vaibhav Pramod Charpe, Ayyakkannu RagupathiKuo Chu Hwang
Journal of the American Chemical Society, 卷.139(8), 頁碼.2896-2899
03/2017

摘要

Catalysis Chemistry (all) Biochemistry Colloid and Surface Chemistry
Direct oxidative coupling of phenols and terminal alkynes was achieved at room temperature by a visible-light-mediated copper-catalyzed photoredox process. This method allows regioselective synthesis of hydroxyl-functionalized aryl and alkyl ketones from simple phenols and phenylacetylene via CC triple bond cleavage. 47 examples were presented. From a synthetic perspective, this protocol offers an efficient synthetic route for the preparation of pharmaceutical drugs, such as pitofenone and fenofibrate.

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